Steam's in-home streaming takes up both devices. When you're moving the mouse and pressing keys on your client (the underpowered laptop), it's sending those same key presses and mouse movents to the host (your gaming PC). Computers don't really respond well/aren't designed to have multiple users in the same desktop environment at the same time.
Another user linked Wolf which uses Docker containers, or you'd need to set up a virtual machine inside your gaming PC that would become the host instead.
Is it possible? Sure.
Is it viable? No.