Okami has a truly beautiful soundtrack, my favourites are the 'The Sun Rises' and The Eight Dog Warriors Theme'. Also Calamari Inkantation from Splatoon is fantastic.
Some great ones:
Gyruss (arcade)
Bubble Bobble (arcade)
WipeOut 2097(XL) (psx - probably the best example of songs that compliment the gameplay)
Afterburner II (arcade - just one specific track called City 202, at time 15:34)
Edit: 2 more
720 ( arcade - blistering)
Rolling Thunder ( arcade - max funky )
Final fantasy 6 Chrono trigger Street fighter 2 Street fighter v Super Mario Bros 3 Mega Man 2 Undertale And this is really unfair but Def Jam fight for New York
For me personally some of my favorites (most memorable) are:
Hitman 2: Silent Assassin main title (and first half of the OST)
Divinity Original Sin 2 main title
Original vanilla WoW main title music
Sanctuary from Borderland 3’s OST
BFG Division from DOOM
Pretty much the entire Skyrim soundtrack
Most of the Witcher 3 soundtrack. My favorite is probably On the Champs-Désolés, which is from the Blood and Wine expansion.
SNES Wild Guns final theme Song
I am personally in love with Far Cry 5's soundtrack.
So many great answers already, but one I don't think I've seen mentioned yet is the soundtrack for Bastion
Probably not when you wrote this but now theres four mentions. 😊
Def hollow knight, I think it captures the essence of a long decaying kingdom perfectly.
Right now I'm going to have to go with a tie between Brok and Graff from Brok the Investigator and the legacy soundtrack piece After The Flames by Josh Woodward from SuperTuxKart.
Personally, Quake (1996). I remember playing it as a teen and actually feeling my heart rate increase with the music. It was the first game that the music really immersed me into the game.
Honorable mention, The Housebuilding Song from RDR2. Just a perfect way to lighten the mood after such a hard hitting chapter.
Unorthodox opinion here but Wasteland 3, the first time the Battle Hymn of the Republic played over a fight was incredible.
Just one track? The Requiem of Shield Knight from Shovel Knight.
Ys
I’ll add two of my favourites that haven’t been mentioned yet - Metroid Prime is my all time favourite and Horizon: Zero Dawn and Forbidden West which I’ve been listening to a ton late lately
Space Invaders
The theme song of Locoroco. Though the lyrics are in a made-up language, I can feel the desire for world peace in this song.
Tunic has an otherworldly soundtrack. It's perfect music to listen to while working. https://youtu.be/nnvjKf_mRYM
I listen to "Carmeaty Burana" from Super Meat Boy all the time.
Pretty much any Danny Baranowsky is gonna be good.
Deep Stone Lullaby fro the Deep Stone Crypt raid in Destiny 2.
It’s an absolutely beautiful piece of music, but so much impactful more when tied to where it appears in the raid as you battle your way across the underside of the space station, all of the other sounds muffled by the vacuum of space.
I don’t know who the guy is, but this video of DrLupo playing it with an orchestra playing the track live while he does is pretty damned amazing.
https://m.youtube.com/watch?v=33ZP8_aAdNI
Kenshi has some of the best ambient music. Scorching wind gives chills every time.
A few i havent seen mentioned.
Sonic 2 and 3 on megadrive. Especially the ice zone with the snowboard on 3. https://youtu.be/hYxlqTpZ-24
Icewind dale. The kuldahar music is epic. https://youtu.be/B92P1-OUNJo or easthaven in peace https://youtu.be/ERd5stTsaBc
There is a reason Touhou has two fandoms, one for its games and the other for its music. The music alone saved it from being another Oregon Trail and eventually got it its own anime.
Really really obscure but I could never take this song off my head, from A Thousand Arms, psx game. Game was a goor jrpg.
Underwater theme from donkey Kong country
It’s not better than Tetris I’ll admit. But I’ve always had a soft spot for the Mass Effect soundtrack.
Ace Combat
Skyrim was pretty epic… even the “wandering around” music was perfect.
But my #1 is Still Alive (closing theme song to Portal).
Not sure about best but the music the black mesa game did for the half life remaster was amazing.
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