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Zrythm Digital Audio Workstation Abandoning GTK For Qt6
(www.phoronix.com)
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It's really rare for a project to completely rewrite to a new toolkit. VLC in circa 2007 did it (moved to Qt - even stole their volume control widget directly from Amarok at the time). GCompris ended up as a KDE project despite originating in Gnome (along with toolkit change, but it weirdly kept the name). LXDE->LXQT also. But I don't actually have that many examples.
audacious too! though oddly enough they've gone back to gtk3 in recent versions alongside their qt version